Tuning the responsivity of monoclinic (InxGa1-x)2O3solar-blind photodetectors grown by metal organic chemical vapor deposition


Hatipoglu İ., Mukhopadhyay P., Alema F., Sakthivel T. S., Seal S., Osinsky A., ...Daha Fazla

Journal of Physics D: Applied Physics, cilt.53, sa.45, 2020 (SCI-Expanded) identifier

  • Yayın Türü: Makale / Tam Makale
  • Cilt numarası: 53 Sayı: 45
  • Basım Tarihi: 2020
  • Doi Numarası: 10.1088/1361-6463/aba313
  • Dergi Adı: Journal of Physics D: Applied Physics
  • Derginin Tarandığı İndeksler: Science Citation Index Expanded (SCI-EXPANDED), Scopus, Academic Search Premier, Aerospace Database, Applied Science & Technology Source, Chemical Abstracts Core, Communication Abstracts, Compendex, Computer & Applied Sciences, INSPEC, Metadex, Civil Engineering Abstracts
  • Anahtar Kelimeler: high responsivity, indium gallium oxide films, metal organic chemical vapor deposition, metal-semiconductor-metal, oxygen vacancies, solar blind photodetector
  • Gazi Üniversitesi Adresli: Hayır

Özet

© 2020 IOP Publishing Ltd.We report on the fabrication and characterization of solar-blind photodetectors based on metal organic chemical vapor deposition grown polycrystalline monoclinic indium gallium oxide (InxGa1-x)2O3 alloys on sapphire using N2O for oxidation. The effects of growth conditions on indium incorporation efficiency and oxygen vacancies of the (InxGa1-x)2O3 alloy, photo-to-dark current ratio (PDR), gain and responsivity of the fabricated photodetectors were investigated. The optical bandgap of the films was found to decrease due to the indium incorporation (x = 20.3%, 17.7%, 10.6% for samples A, B, and C, respectively) into the lattice of gallium oxide. By increasing the indium content incorporated into the lattice of Ga2O3, we demonstrated solar-blind photodetectors whose peak responsivity increased from 0.79 A/W (Ga2O3) to 319.1 A/W, 66.1 A/W and 27.7 A/W for samples A, B and C, respectively at 5 V applied bias with the cut off wavelength below 280 nm. Increasing in content resulted in a higher concentration of oxygen vacancies in as-grown films. Increased oxygen vacancies as a result of the change in growth conditions lead to higher photoconductive gain, higher responsivities, and lower PDR, demonstrating a trade-off between responsivity and the PDR. To the best of our knowledge, the peak responsivity value reported in this work is the highest for (InxGa1-x)2O3 based solar-blind photodetectors. Fast rise and fall times in the order of 100 ms have been measured for the photodetectors.