Dielectric properties of Ag/Ru-0.03-PVA/n-Si structures


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Badali Y., Kocyigit S., USLU İ., ALTINDAL Ş.

BULLETIN OF MATERIALS SCIENCE, vol.42, no.5, 2019 (SCI-Expanded, Scopus)

  • Publication Type: Article / Article
  • Volume: 42 Issue: 5
  • Publication Date: 2019
  • Doi Number: 10.1007/s12034-019-1875-4
  • Journal Name: BULLETIN OF MATERIALS SCIENCE
  • Journal Indexes: Science Citation Index Expanded (SCI-EXPANDED), Scopus
  • Keywords: Ag/Ru-0.03-PVA/n-Si, impedance spectroscopy, frequency dependence, surface states, AC ELECTRICAL-CONDUCTIVITY, IONIC-LAYER ADSORPTION, THIN-FILMS, SPECTROSCOPY, RELAXATION, FREQUENCY, RU
  • Open Archive Collection: AVESIS Open Access Collection
  • Gazi University Affiliated: Yes

Abstract

Ag/Ru-0.03-PVA/n-Si structures were successfully prepared and their morphological and electrical properties were investigated. The obtained electrical results suggested that the complex dielectric constant (epsilon* = epsilon'-j epsilon ''), complex electric modulus M* = M' + jM ''', loss tangent (tan delta) and alternating current (ac) electrical conductivity (sigma(ac)) are all a strong function of the frequency (f) and applied voltage. The changes in these parameters are the results of the existence of the surface states (N-ss) or interface traps (D-it = N-ss), interfacial polymer layer, surface and dipole polarizations and hopping mechanisms. The values of epsilon' and epsilon '' show a steep decline with increasing frequency and then reach a constant value at high frequency, whereas the increments of M' and M '' with frequency are exponential. The tan delta vs. log f plot has a strong peak behaviour, especially in the accumulation region. These experimental results suggested that the Ru-0.03-PVA interfacial layer could be used as a high dielectric material instead of conventional materials.